The arsenic‐bearing copper-gold concentrate produced by the beneficiation plant of a Chilean mine was treated using a single direct cyanidation method, with gold and silver leaching rates of 83.86 % and 76.19 %, respectively, while copper could not be effectively recovered. The use of roasting-acid leaching-cyanidation resulted in gold and silver leaching rates of 94.20 % and 81.98 %, respectively, and a copper leaching rate of 83.38 %. However, the recovery of gold, silver, and copper still needs to be improved. Through systematic experiments, the process flow is finalized, which involves enhanced cyanide leaching for gold and silver, flotation recovery of copper from cyanide tailings, two‐stage roasting, acid leaching to recover copper, and cyanide leaching of acid leaching residues for gold and silver. The comprehensive recovery rates for gold, silver, and copper reach 98.95 %, 97.90 %, and 92.41 %, respectively. This process achieves efficient comprehensive recovery of valuable elements from difficult‐to‐process arsenic‐bearing copper-gold concentrates and can serve as a reference for the sorting and recovery of such types of gold concentrates.